Publications (PR)

133) Single molecule FRET analysis of the 11 Discrete steps of a DNA actuator. Hildebrandt, L. L.; Preus, S.; Zhang, Z.; Voigt, N. V.; Gothelf, K. V., Birkedal, V. J. Am. Chem. Soc. 2014, DOI: 10.1021/ja502580t
132) Singlet Oxygen of homochiral tris-indanyl molecular rodsKjeldsen, N. D.; Funder, E. D.; Gothelf, K. V. Org. Biomol. Chem. 2014, 12, 3679-3685
131) Singlet oxygen in DNA nanotechnologyTørring, T.; Helmig, S. D.; Ogilby, P. R.; Gothelf. K. V. Acc. Chem. Res. 2014, DOI: 10.1021/ar500034y
130) Tailoring on-surface supramolecular architectures based on adenine directed self-assemblyTan, Q.; Zhang, C.; Wang, N.; Sun, Q.; Jacobsen, M. F.; Gothelf, K. V.; Besenbacher, F.; Hu, A.; Xu, W. Chem. Comm. 2014, 50, 356-358. DOI: 10.1039/c3cc46149a
129) Efficient colorimetric and fluorescent detection of fluoride in DMSO-water mixtures with arylaldoximesRosen, C. B.; Hansen, D. J.; Gothelf, K. V. Org. Biomol. Chem. 2013, 11, 7916-7922. DOI: 10.1039/c3ob41078a
128) Isothermal Hybridization Kinetics of DNA Assembly of Two-Dimensional DNA Origami. Song, J.; Zhang, Z.; Zhang, S.; Liu, L.; Li, Q.; Xie, E. Q.; Gothelf, K. V.; Besenbacher, F.; Dong, M. Small. 2013, 9, 2954-2959. DOI: 10.1002/smll.201202861
127) Self-Assembly of DNA Origami and Single-Stranded Tile Structures atRoom Temperature. Zhang, Z.; Song, J.; Besenbacher, F.; Dong, M.; Gothelf, K. V.Angew. Chem. Int. Ed. 2013, 52, 9219. DOI: 10.1002/anie.201303611
126) Electron-induced damage of biotin studied in the gas phase and in the condensed phase at a single-molecule level. Keller, A.; Kopyra, J.; Gothelf, K. V.; Bald, I. New J. Phys. 2013, 15, no. 083045, DOI: 10.1088/1367-2630/15/8/083045
125) Enzymatic Ligation of Large Biomolecules to DNA. Sørensen, R. S.; Okholm, A. H.; Schaffert, D.; Kodal, A. L. B.; Gothelf, K. V.; Kjems. J. ACS Nano, 2013, 7, 8098-8104. DOI: 10.1021/nn403386f
124) A DNA-tweezer-actuated enzyme nanoreactor. Liu, M.; Fu, J.; Hejesen, C.; Yang, Y.; Woodbury, N. W.; Gothelf, K. V.; Liu, Y.;Yan, H. Nat. Comm. 2013, 4, no. 2127, DOI: 10.1038/ncomms3127
123) DNA Nanotechnology: A Curiosity or a Promising Technology?Tørring, T; Gothelf, K. V. F100Prime Rep. 2013, 5, DOI: 10.12703/P5-14
122) Oligo(naphthylene-ethynylene) Molecular Rods. Cramer, J. R.; Ning, Y. X.; Shen, C.; Nuermaimaiti, A.; Besenbacher, F.; Linderoth, T. R.; Gothelf, K. V. Eur. J. Org. Chem. 2013, 2813-2822. DOI: 10.1002/ejoc.201201752
121) On Electrogenerated Acid-Facilitated Electrografting of Aryltriazenes to Create Well-Defined Aryl-Tethered Films. Vinther, J.; Iruthayaraj, J.; Gothelf, K. V.; Pedersen, S. U.; Daasbjerg, K. Langmuir, 2013, 29, 5181–5189
120) On-Surface Azide–Alkyne Cycloaddition on Cu(111): Does It “Click” in Ultrahigh Vacuum? Bebensee, F.; Bombis, C.; Vadapoo, S.-R. Cramer, J. R.; Besenbacher, F.; Gothelf, K. V.; Linderoth, T. R.J. Am. Chem. Soc., 2013, 135, 2136–2139.
119) Novel Self-Assembled Nanoparticles of Testosterone-Modified Glycol Chitosan and Fructose Chistosan for Controlled Release. Perez Quinones, J.; Gothelf, K. V.; Kjems, J.; Heras, A.; Schmidt, C.; Peniche, C. J Biomater. Tissue Eng. 2013, 3, 164-172, DOI: 10.1166/jbt.2013.1071
118) Self-assembled Nanoparticles of Modified-Chitosan Conjugates for the Sustained Release of DL-alpha-tocopherol. Perez Quinones, J.; Gothelf, K. V.; Kjems, J.; Yang, C.; Caballero, A. M. H.; Schmidt C.; Covas, C. P. Carbohydr. Polym. 2013, 92, 856-864, DOI: 10.1016/j.carbpol.2012.10.005
117) Single-step rapid assembly of DNA origami nanostructures for addressable nanoscale bioreactors. Fu, Y.;, Zeng, D.; Chao, J.;, Zhang, Z.; Liu, H.; Ma, H.; Huang, Q.; Gothelf, K.; Fan, C. J. Am. Chem. Soc. 2013 135, 696-702.
116) N,06-partially acetylated chitosan nanoparticles hydrophobically-modified for controlled release of steroids and vitamin E. Pérez Quinones, J.; Gothelf, K. V.; Kjems.; Caballero, A. M. H.; Schmidt, C.; Covas, C. P. Carbohyd. Polym. 2013, 91, 143-151, DOI: 10.1016/j.carbpol.2012.07.080
115) A traceless aryl-triazene linker for DNA-directed chemistryHejesen, C.; Petersen, L. K.; Hansen, N. J. V.; Gothelf. K. V. Org. Biomol. Chem. 2013, 11, 2493-2497.
114) Transfer of a protein pattern from self-assembled DNA origami to a functionalized substrate. Katerina Busuttil, Alexandru Rotaru, Mingdong Dong, Flemming Besenbacher and Kurt V. Gothelf Chem. Commun., 2013, 49, 1927-1929.
113) RNA Aptamer-Based Electrochemical Biosensor for Selective and Label-Free Analysis of Dopamine. Farjami, E.; Nielsen, J.; Gothelf, K.; Kjems, J.; Ferapontova, E. Anal. Chem. 2013 85, 121-128.
112) Steering Supramolecular patters by nucleobase-terminated molecules. Shen, C: Cramer, J. R.: Jacobsen, M. F.; Liu, L.; Zhang, S.; Dong, M.; Gothelf, K. V.; Besenbacher, F. Chem. Commun. 2013 49, 508-510.
111) Extended DNA Tile Actuators. Kristiansen, M.; Kryger, M. B. L.; Zhang, Z.; Voigt, N. V.; Birkedal,V. Gothelf, K. V. ChemPlusChem 2012, 77, 636–642.
110) Electrochemical sandwich assay for attomole analysis of DNA and RNA from beer spoilage bacteria Lactobacillus brevis. Shipovskov, S.; Saunders, A. M.; Nielsen, J. S.;Hansen, M. H.; Gothelf, K. V.; Ferapontova, E. E.; Biosensors & Bioelectronics 2012, 37, 99-106
109) Increased anticoagulant activity of thrombin-binding DNA aptamers by nanoscale organization on DNA nanostructures. Rangnekar, A.; Zhang, A. M.; Li, S. S.; Bompiani, K. M.; Hansen, M. N.; Gothelf, K. V.; Sullenger, B. A.; LaBean, T. H. Nanomed-Nanotechnol. 2012, 8, 673-681.
108) Direct Visualization of Transient Thermal Response of a DNA Origami. Song, J.; Arbona, J. M. ; Zhang, Z.; Liu, L.; Xie, E.Q.; Elezgaray, J.; Aime, J. P.; Gothelf, K.V.; Besenbacher, F.; Dong, M. D. J. Am. Chem. Soc. 2012, 134, 9844-9847
107) Self-Assembled Nanoparticles of Glycol Chitosan – Ergocalciferol Succinate conjugate, for controlled release. Quinones Pérez, J.; Gothelf , K. V.; Kjems, J.; Caballero, A. M. H.; Scmidt, C.; Covas, C. P. Carbohyd. Polym. 2012, 88, 1373-1377. DOI: 10.1016/j.carbpol.2012.02.039
106) Probing electron-induced bond cleavage at the single-molecule level using DNA origami templates. Keller, A.; Bald, I.; Rotaru, A.; Cauët, E.; Gothelf, K. V.; Besenbacher, F. ACS Nano, 2012, 6, 4392-4399.
105) Synthesis of Dopamine and Serotonin Derivatives for Immobilization on a Solid Support. Funder, E. D.; Jensen, A. B.; Tørring, T.;   Kodal, A. L. B.; Azcargorta, A. R.; Gothelf, K. V. J. Org. Chem. 2012, 77, 3134–3142
104) Multilayer DNA Origami Packed on Hexagonal and Hybrid Lattices. Ke, Y.; Voigt, N. V.; Gothelf, K. V.; Shih, W. M. J. Am. Chem. Soc. 2012, 134, 1770−1774.
103) DNA-programmed Glaser-Eglinton reactions for the synthesis of conjugated molecular wires. Ravnsbæk, J. B.; Jacobsen, M. F.; Rosen, C. B.; Voigt, N. V.; Gothelf, K. V. Angew. Chem. Int. Ed. 2011, 50, 10851–10854.
102) Chiral induction by seeding surface assemblies of chiral switchesMasini, F.; Kalashnyk, N.; Knudsen, M. M.; Cramer, J. R.; Lægsgaard, E.; Besenbacher, F.; Gothelf, K. V.; Linderoth, T. R. J. Am. Chem. Soc. 2011, 7, 13910–13913.
101) Control of self-assembled 2D nanostructures by methylation of guanineBald, I.; Wang, Y.-g.; Dong, M.; Rosen, C. B.; Ravnsbæk, J. B.; Zhuang, G.- l.; Gothelf, K. V.; Wang, J.-g.; Besenbacher, F., Small 2011, 7, 939–949.
100) Single molecule microscopy methods for the study of DNA origami structuresBirkedal, V.; Dong, M.; Golas, M. M.; Sander, B.; Andersen, E. S.; Gothelf, K. V.; Besenbacher, F.; Kjems, J. Microscopy Research and Technique 2011, 74, 688–698.
99) “Off–On” electrochemical hairpin-DNA-based genosensor for cancer diagnosticsFarjami, E.; Clima, L.; Gothelf, K. V.; Ferapontova, E. E. Anal. Chem. 2011, 83, 1594–1602.
98) Recent advances in electrochemical aptamer-based sensorsFerapontova, E. E.; Gothelf, K. V. Curr. Org. Chem. 2011, 15, 498–505.
97) β-olefination of 2-alkynoates leading to trisubstituted 1,3-dienesJacobsen, M. J.; Funder, E. D.; Cramer, J. R.; Gothelf, K. V. Org. Lett. 2011, 13, 3418–3421.
96) Site-specific chemical labeling of long RNA moleculesJahn, K.; Olsen, E. M.; Nielsen, M. M.; Tørring, T.; MohammadZadegan, R.; Andersen, E. S.; Gothelf, K. V.; Kjems, J. Bioconjugate Chem. 2011, 22, 95–100.
95) Functional patterning of DNA origami by parallel enzymatic modificationJahn, K.; Tørring, T.; Voigt, N. V.; Sørensen, R. S.; Kodal, A. L. B.; Andersen, E. S.; Gothelf, K. V.; Kjems, J. Bioconjugate Chem. 2011, 22, 819–823.
94) Controlling chiral organization of molecular rods on Au(111) by molecular designKnudsen, M. K.; Kalashnyk, N.; Masini, F.; Cramer, J. R.; Lægsgaard, E.; Besenbacher, F.; Linderoth, T. R.; Gothelf., K. V. J. Am. Chem. Soc. 2011, 133, 4896–4905.
93) Combining aryltriazenes and electrogenerated acids to create well-defined aryl-tethered films and patterns on surfacesKongsfelt, M.; Vinther, J.; Malmos, K.; Ceccato, M.; Torbensen, K.; Knudsen, C. S.; Gothelf, K. V.; Pedersen, S. U.; Daasbjerg, K. J. Am. Chem. Soc. 2011, 133, 3788–3791.
92) Design and construction of double-decker tile as a route to three-dimensional periodic assembly of DNAMajumder, U.; Rangnekar, A.; Gothelf, K. V.; Reif, J. H.; LaBean, T. H. J. Am. Chem. Soc. 2011, 133, 3843–3845.
91) Development of a lipase-based optical assay for detection of DNAPinijsuwan, S.; Shipovskov, S.; Surareungchai, W.; Ferapontova, E. E.; Gothelf, K. V. Org. Biomol. Chem. 2011, 9, 6352–6356
90) Design and synthesis of DNA four-helix bundlesRangnekar, A.; Gothelf, K. V.; LaBean, T. H. Nanotechnology 2011, 22, 235601.
89) DNA origami: a quantum leap for self-assembly of complex structuresTørring, T.; Voigt, N. V.; Nangreave, J.; Yan, H.; Gothelf, K. V. Chem. Soc. Rev. 2011, 40, 5636-5646.
88) A DNA tile actuator with eleven discrete statesZhang, Z.; Olsen, E. M.; Kryger, M.; Voigt, N. V.; Tørring, T.; Gültekin, E.; Nielsen, M.; MohammadZadegan, R.; Andersen, E. S.; Nielsen, M. M.; Kjems, J.; Birkedal, V.; Gothelf, K. V. Angew. Chem. Int. Ed. 2011, 50, 3983–3987.
87) A nucleic acid dependent chemical photocatalysis in live human cellsArian, D.; Cló, E.; Gothelf, K. V.; Mokhir, A. Chem,. Eur. J. 2010, 16, 288–295.
86) Steering organizational and conformational surface chirality by controlling molecular chemical functionalityBombis, C.; Weigelt, S.; Knudsen, M. M.; Nørgaard, M.; Busse, C.; Lægsgaard, E.; Besenbacher, F.; Gothelf, K. V.; Linderoth, T. R., ACS Nano 2010, 4, 297–311.
85) DNA interactions with a methylene blue redox indicator depend on the DNA length and are sequence specificFarjami, E.; Clima, L.; Gothelf, K. V.; Ferapontova, E. E. Analyst 2010, 135, 1443–1448.
84) Electrochemical DNA sandwich assay with a lipase label for attomole detection of DNAFerapontova, E. E.; Hansen, M. N.; Saunders, A. M.; Shipovskov, S.; Sutherland, D. S.; Gothelf, K. V. Chem. Commun. 2010, 46, 1836–1838.
83) Synthesis and application of a triazene–ferrocene modifier for immobilization and characterization of oligonucleotides at electrodesHansen, M. N.; Farjami, E.; Kristiansen, M.; Clima, L.; Pedersen, S. U.; Daasbjerg, K.; Ferapontova, E. E.; Gothelf, K. V. J. Org. Chem. 2010, 75, 2474–2481.
82) Weave tile architecture construction strategy for DNA nanotechnologyHansen, M. N.; Zhang, A. M.; Rangnekar, A.; Bompiani, K. M.; Carter, J. D.; Gothelf, K. V.; LaBean, T. H. J. Am. Chem. Soc. 2010, 132, 14481–14486.
81) Single molecule atomic force microscopy studies of photosensitized singlet oxygen behavior on a DNA origami templateHelmig, S.; Rotaru, A.; Arian, D.; Kovbasyuk, L.; Arnbjerg, J.; Ogilby, P. R.; Kjems, J.; Mokhir, A.; Besenbacher, F.; Gothelf, K. V. ACS Nano 2010, 4, 7475–7480.
80) Small molecule induced control in duplex and triplex DNA-directed chemical reactionsJacobsen, M. F.; Ravnsbæk, J. B.; Gothelf, K. V. Org. Biomol. Chem. 2010, 8, 50–52.
79) DNA-templated covalent coupling of G4 PAMAM dendrimersLiu, H.; Tørring, T.; Dong, M.; Rosen, C. B.; Besenbacher, F.; Gothelf, K. V. J. Am. Chem. Soc. 2010, 132, 18054–18056.
78) Selective dsDNA-templated formation of copper nanoparticles in solutionRotaru, A.; Dutta, S.; Jentzsch, E.; Gothelf, K. V.; Mokhir, A. Angew. Chem. Int. Ed. 2010, 49, 5665–5667.
77) DNA nanotechnology: Steps towards automated synthesisRotaru, A.; Gothelf, K. V. Nat. Nanotech. 2010, 5, 760–761.
76) A novel secondary DNA binding site in human topoisomerase I unravelled by using a 2D DNA origami platformSubramani, R.; Juul, S.; Rotaru, A.; Andersen, F. F.; Gothelf, K. V.; Mamdouh, W.; Besenbacher, F.; Dong, M.; Knudsen, B. R. ACS Nano 2010, 4, 5969–5977.
75) Reversible pH-regulated control of photosensitized singlet oxygen production using a DNA i-motifTørring, T.; Toftegaard, R.; Arnbjerg, J.; Ogilby, P. R.; Gothelf, K. V. Angew. Chem. Int. Ed. 2010, 49, 7923–7925.
74) Single-molecule chemical reactions on DNA origamiVoigt, N. V.; Tørring, T.; Rotaru, A.; Jacobsen, M. F.; Ravnsbæk, J. B.; Subramani, R.; Mamdouh, W.; Kjems, J.; Mokhir, A.; Besenbacher, F.; Gothelf, K. V. Nat. Nanotech. 2010, 5, 200.
73) Supramolecular porous network formed by molecular recognition between chemically modified nucleobases guanine and cytosineXu, W.; Wang, J.-g.; Jacobsen, M. F.; Mura, M.; Yu, M.; Kelly, R. E. A.; Meng, Q.-q.; Lægsgaard, E.; Stensgaard, I.; Linderoth, T. R.; Kjems, J.; Kantorovich, L. N.; Gothelf, K. V.; Besenbacher, F. Angew. Chem. Int. Ed. 2010, 49, 9373–9377.
72) Synthesis of functional molecular rod oligomersAndersen, C. S.; Gothelf, K. V. Org. Biomol. Chem. 2009, 7, 58–60.
71) Distance dependent interhelical couplings of organic rods incorporated in DNA 4-helix bundlesAndersen, C. S.; Knudsen, M. M.; Chhabra, R.; Liu, Y.; Yan, H.; Gothelf, K. V. Bioconjugate Chem. 2009, 20, 1538–1546.
70) Self-assembly of a nanoscale DNA box with a controllable lidAndersen, E. S.; Dong, M.; Nielsen, M. M.; Jahn, K.; Subramani, R.; Mam- douh, W.; Golas, M. M.; Sander, B.; Stark, H.; Oliveira, C. L. P.; Pedersen, J. S.; Birkedal, V.; Besenbacher, F.; Gothelf, K. V.; Kjems, J. Nature 2009, 459, 73–76.
69) Optimization of the electrochemical RNA-aptamer based biosensor for theophylline by using a Methylene Blue redox labelFerapontova, E. E.; Gothelf, K. V. Electroanalysis 2009, 21, 1261–1266.
68) Effect of serum on an RNA aptamer-based electrochemical sensor for theophyllineFerapontova, E. E. ; Gothelf, K. V. Langmuir 2009, 25, 4279–4283.
67) A yoctoliter-scale DNA reactor for small-molecule evolutionHansen, M. H.; Blakskjær, P.; Petersen, L. K.; Hansen, T. H.; Højfeldt, J. W.; Gothelf, K. V.; Hansen, N. J. V. J. Am. Chem. Soc. 2009, 131, 1322–1327.
66) Synthesis and electrochemical studies of an anthraquinone-conjugated nucleoside and derived oligonucleotidesJacobsen, M. F.; Ferapontova, E. E.; Gothelf, K. V. Org. Biomol. Chem. 2009, 7, 905–908.
65) Effect of polymer cross-links on oxygen diffusion in glassy PMMA filmsKlinger, M.; Tolbod, L. P.; Gothelf, K. V.; Ogilby, P. R. ACS Appl. Mater. Interfaces 2009, 1, 661–667.
64) Self-assembly of artificial nucleobase 1H-benzimidazole-4,7-dione at the liquid/solid interfaceMamdouh, W.; Kelly, R. E. A.; Dong, M.; Jacobsen, M. F.; Ferapontova, E. E.; Kantorovich, L. N.; Gothelf, K. V.; Besenbacher, F. J. Phys. Chem. B 2009, 113, 8675–8681.
63) Bridging one helical turn in double-stranded DNA by templated dimerization of molecular rodsAndersen, C. S.; Yan, H.; Gothelf, K. V. Angew. Chem. Int. Ed. 2008, 47, 5569–5572.
62) DNA origami design of dolphin-shaped structures with flexible tailsAndersen, E. S.; Dong, M.; Nielsen, M. M.; Jahn, K.; Lind-Thomsen, A.; Mamdouh, W.; Gothelf, K. V.; Besenbacher, F.; Kjems, J. ACS Nano 2008, 2, 1213–1218.
61) Labeling of DNA via rearrangement of s-2-aminoethyl phosphorothioates to n-(2-mercaptoethyl)phosphoramidatesChen, M.; Gothelf, K. V. Org. Biomol. Chem. 2008, 6, 908–911.
60) An RNA aptamer-based electrochemical biosensor for detection of theophylline in serumFerapontova, E. E.; Olsen, E. M.; Gothelf, K. V. J. Am. Chem. Soc. 2008, 130, 4256–4258.
59) Toward reliable gold nanoparticle patterning on self-assembled DNA nanoscaffoldSharma, J.; Chhabra, R.; Andersen, C. S.; Gothelf, K. V.; Yan, H.; Liu, Y. J. Am. Chem. Soc. 2008, 130, 7820–7821.
58) Molecular self-assembly from building blocks synthesized on a surface in ultrahigh vacuum: Kinetic control and topo-chemical reactionsWeigelt, S.; Bombis, C.; Busse, C.; Knudsen, M. M.; Gothelf, K. V.; Lægsgaard, E.; Besenbacher, F.; Linderoth, T. R. ACS Nano 2008, 2, 651–660.
57) Surface synthesis of 2D branched polymer nanostructuresWeigelt, S.; Busse, C.; Bombis, C.; Knudsen, M. M.; Gothelf, K. V.; Lægsgaard, E.; Besenbacher, F.; Linderoth, T. R. Angew. Chem. Int. Ed. 2008, 47, 4406–4410.
56) Chiral ordering and conformational dynamics for a class of oligo-phenylene-ethynylenes on Au(111)Busse, C.; Weigelt, S.; Petersen, L.; Lægsgaard, E.; Besenbacher, F.; Linderoth, T. R.; Thomsen, A. H.; Nielsen, M.; Gothelf, K. V. J. Phys. Chem. B. 2007, 111, 5850–5860.
55) Rearrangement of s-(2-aminoethyl) thiophosphates to n-(2-mercaptoethyl)phosphoramidatesChen, M.; Maetzke, A.; Knak Jensen, S. J.; Gothelf, K. V. Eur. J. Org. Chem. 2007, 5826–5833.
54) Control and selectivity of photosensitized singlet oxygen production: Challenges in complex biological systemsCló, E.; Snyder, J. W.; Ogilby, P. R.; Gothelf, K. V. ChemBioChem 2007, 8, 475–481.
53) An electrochemical sensor based on the human estrogen receptor ligand binding domainHansen, J. A.; Sumbayev, V. V.; Gothelf, K. V. Nano Lett. 2007, 7, 2831–2834.
52) Synthesis of rigid homo- and heteroditopic nucleobase-terminated molecules incorporating adenine and/or thymineJacobsen, M. F.; Andersen, C. S.; Knudsen, M. M.; Gothelf, K. V. Org. Lett. 2007, 9, 2851–2854.
51) Model systems for activation of nucleic acid encoded prodrugsJacobsen, M. F.; Cló, E., Mokhir, A.; Gothelf, K. V. ChemMedChem 2007, 2, 793–799.
50) Covalent interlinking of an aldehyde and an amine on a Au(111) surface in ultrahigh vacuumWeigelt, S.; Busse, C.; Bombis, C.; Knudsen, M. M.; Gothelf, K. V.; Strunskus, T.; Wöll, C.; Dahlbom, M.; Hammer, B.; Lægsgaard, E.; Besenbacher, F.; Linderoth, T. R. Angew. Chem. Int. Ed. 2007, 46, 9227–9230.
49) Influence of molecular geometry on the adsorption orientation for oligophenylene-ethynylenes on Au(111)Weigelt, S.; Busse, C.; Nielsen, M.; Gothelf, K. V.; Lægsgaard, E.; Besenbacher, F.; Linderoth, T. R. J. Phys. Chem. B 2007, 111, 11342–11345.
48) Synthesis of an elongated linear oligo(phenylene ethynylene)-based building block for application in DNA-programmed assemblyBlakskjær, P.; Gothelf, K. V. Org. Biomol. Chem. 2006, 4, 3442–3447.
47) DNA-programmed control of photosensitized singlet oxygen productionCló, E.; Snyder, J. W.; Voigt, N. V.; Ogilby, P. R.; Gothelf, K. V. J. Am. Chem. Soc. 2006, 128, 4200–4201.
46) Femtomolar electrochemical detection of DNA targets using metal sulfide nanoparticlesHansen, J. A.; Mukhopadhyay, R.; Hansen, J. Ø.; Gothelf, K. V. J. Am. Chem. Soc. 2006, 128, 3860–3861.
45) Quantum-dot/aptamer-based ultrasensitive multi-analyte electrochemical biosensorHansen, J. A.; Wang, J.; Kawde, A.-N.; Xiang, Y.; Gothelf, K. V.; Collins, G. J. Am. Chem. Soc. 2006, 128, 2228–2229.
44) A cleavable amino-thiol linker for reversible linking of amines to DNAHøjfeldt, J. W.; Blakskjær, P.; Gothelf, K. V. J. Org. Chem. 2006, 71, 9556–9557.
43) Efficient N-arylation and N-alkenylation of the five DNA/RNA nucleobasesJacobsen, M. F., Knudsen, M. M.; Gothelf, K. V. J. Org. Chem. 2006, 71, 9183–9190.
42) Chiral switching by spontaneous conformational change in adsorbed organic moleculesWeigelt, S.; Busse, C.; Petersen, L.; Rauls, E.; Hammer, B.; Gothelf, K. V.; Besenbacher, F.; Linderoth, T. R. Nature Mater. 2006, 5, 112–117.
41) Effect of water on the palladium-catalyzed amidation of aryl bromidesDallas, A. S.; Gothelf, K. V. J. Org. Chem. 2005, 70, 3321–3323.
40) A modular approach to DNA-programmed self-assembly of macromolecular nanostructuresGothelf, K. V.; Brown, R. S. Chem. Eur. J. 2005, 11, 1062–1069.
39) DNA-programmed assembly of nanostructuresGothelf, K. V.; LaBean, T. H. Org. Biomol. Chem. 2005, 3, 4023–4037.
38) Preparation temperature dependence of size and polydispersity of alkylthiol monolayer protected gold clustersJørgensen, J. M.; Erlacher, K.; Pedersen, J. S.; Gothelf, K. V Langmuir 2005, 21, 10320–10323.
37) Electrochemical properties of mixed self-assembled monolayers on gold electrodes containing mercaptooctylhydroquinone and alkylthiolsLarsen, A. G.; Gothelf, K. V. Langmuir 2005, 21, 1015–1021.
36) Two-photon photosensitized production of singlet oxygen: Sensitizers with phenylene-ethynylene-based chromophoresMcIlroy, S. P.; Cló, E.; Nikolajsen, L.; Frederiksen, P. K.; Nielsen, C. B.; Mikkelsen, K. V.; Gothelf, K. V.; Ogilby, P. R. J. Org. Chem. 2005, 70, 1134–1146.
35) DNA-directed coupling of organic modules by multiple parallel reductive aminations and subsequent cleavage of selected DNA sequencesNielsen, M.; Dauksaite, V.; Kjems, J.; Gothelf, K. V. Bioconjugate Chem. 2005, 16, 981–985.
34) Formation and structure of conjugated salen-cross-linked polymers and their application in asymmetric heterogeneous catalysisNielsen, M. M.; Thomsen, A. H.; Jensen, T. R.; Jakobsen, H. J.; Skibsted, J.; Gothelf, K. V. Eur. J. Org. Chem. 2005, 2005, 342–347.
33) Self-assembly of aluminium-salen coupled nanostructures from encoded modules with cleavable disulfide DNA-linkersBrown, R. S.; Nielsen, M.; Gothelf, K. V. Chem. Commun. 2004, 1464–1465.
32) Modular DNA-programmed assembly of linear and branched conjugated nanostructuresGothelf, K. V.; Thomsen, A.; Nielsen, M.; Cló, E.; Brown, R. S. J. Am. Chem. Soc. 2004, 126, 1044–1046.
31) An electrochemical quartz crystal microbalance study of the etching of gold surfaces in the presence of tetramethylthioureaLarsen, A. G.; Johannsen, K.; Gothelf, K. V. J. Coll. Int. Sci. 2004, 279, 158–166.
30) Synthesis of linear and tripoidal oligo(phenylene ethynylene)-based building blocks for application in modular DNA-programmed assemblyNielsen, M.; Thomsen, A. H.; Cló, E.; Kirpekar, F.; Gothelf, K. V. J. Org. Chem. 2004, 69, 2240–2250.
29) Catalytic asymmetric Henry reactions of silyl nitronates with aldehydesRisgaard, T.; Gothelf, K. V.; Jørgensen, K. A. Org. Biomol. Chem. 2003, 1, 153–156.
28) Nucleophilic addition of nitrones to ketones: Development of a new catalytic asymmetric nitrone-aldol reactionBøgevig, A.; Gothelf, K. V.; Jørgensen, K. A. Chem. Eur. J. 2002, 8, 5652–5661.
27) Catalytic asymmetric 1,3-dipolar cycloaddition reactions of azomethine ylides – a simple approach to optically active highly functionalized proline derivativesGothelf, A. S.; Gothelf, K. V.; Hazell, R. G.; Jørgensen, K. A. Angew. Chem. Int. Ed. 2002, 41, 4236–4238.
26) Attachment of alkyltrichlorosilanes to the terminal 3,5-dihydroxyphenyl moiety of a self-assembled thiol monolayer on goldGothelf, K. V.; Larsen, A. G. J. Coll. Int. Sci. 2002, 255, 356–362.
25) Electron transfer reactions of self- assembled monolayers of thio(phenylacetylene)n-substituted chiral metal-salen complexesNielsen, M.; Larsen, N. B.; Gothelf, K. V. Langmuir 2002, 18, 2795–2799.
24) Density functional theory study of enantiospecific adsorption at chiral surfacesSljivancanin, Z.; Gothelf, K. V.; Hammer, B. J. Am. Chem. Soc. 2002, 124, 14789–14794.
23) The first catalytic asymmetric Aza-Henry reaction of nitronates with imines: A novel approach to optically active β-nitro-α-amino acid- and α,β-diamino acid derivativesKnudsen, K. R.; Risgaard, T.; Nishiwaki, N.; Gothelf, K. V.; Jørgensen, K. A. J. Am. Chem. Soc. 2001, 123, 5843–5844.
22) Synthesis and catalytic properties of p-acylthio(phenylacetylene)n substituted chiral manganese salen complexesNielsen, M.; Gothelf, K. V. J. Chem. Soc., Perkin Trans. 1 2001, 2440–2444.
21) Catalytic enantioselective addition of nitro compounds to imines – a simple approach for the synthesis of optically active β-nitro-α-amino estersNishiwaki, N.; Rahbek Knudsen, K.; Gothelf, K. V.; Jørgensen, K. A. Angew. Chem. Int. Ed. 2001, 40, 2992–2995.
20) Self-assembled monolayers of long-chain xanthic acids on gold studied by voltammetryGothelf, K. V. J. Electroanal. Chem. 2000, 494, 147–150.
19) Catalytic enantioselective 1,3-dipolar cycloaddition reactions of nitronesGothelf, K. V., Jørgensen, K. A. Chem. Commun. 2000, 1449–1458. Feature Article.
18) Catalytic enantioselective inverse-electron demand 1,3-dipolar cycloaddition reactions of nitrones with alkenesSimonsen, K. B.; Bayón, P.; Hazell, R. G.; Gothelf, K. V.; Jørgensen, K. A. J. Am. Chem. Soc. 1999, 121, 3845–3853.
17) Molecular sieve dependent absolute stereoselectivity in asymmetric catalytic 1,3-dipolar cycloaddition reactionsGothelf, K. V.; Hazell, R. G.; Jørgensen, K. A. J. Org. Chem. 1998, 63, 5483–5488.
16) Asymmetric 1,3-Dipolar cycloaddition reactionsGothelf, K. V.; Jørgensen, K. A. Chem. Rev. 1998, 98, 863–910.
15) A simple synthetic approach to 3,3’-diaryl BINOLsSimonsen, K. B.; Gothelf, K. V.; Jørgensen, K. A. J. Org. Chem. 1998, 63, 7536–7538.
14) On the structure of C,N-diphenylnitrone in 1,3-dipolar cycloaddition reactionsGothelf, K. V.; Hazell, R. G.; Jørgensen, K. A. Acta Chem. Scand. 1997, 51, 1234–1235.
13) On the trans-cis controversy in Ti-TADDOLate-catalysed cycloadditions. Experimental indications for the structure of the reactive catalyst-substrate intermediateGothelf, K. V.; Jørgensen, K. A. J. Chem. Soc., Perkin Trans. 2 1997, 111–116.
12) Improvement of TADDOLate-TiCl2-catalyzed 1,3-dipolar nitrone cycloaddition reactions by substitution of the oxazolidinone auxiliary of the alkene with succinimideJensen, K. B.; Gothelf, K. V.; Hazell, R. G.; Jørgensen, K. A. J. Org. Chem. 1997, 62, 2471–2477.
11) Control of regio-, diastereo-, and enantioselectivity in the [Ti(OTs)2(TADDOLato)]-catalyzed 1,3-dipolar cycloaddition reaction between 3-acryloyloxazolidin-2-one and nitronesJensen, K. B.; Gothelf, K. V.; Jørgensen, K. A. Helv. Chim. Acta 1997, 80, 2039–2046.
10) Lanthanide-catalyzed endo- and enantioselective 1,3-dipolar cycloaddition reactions of nitrones with alkenesSanchez-Blanco, A. I.; Gothelf, K. V.; Jørgensen, K. A. Tetrahedron Lett. 1997, 38, 7923–7926.
9) Control of diastereo- and enantioselectivity in metal-catalyzed 1,3-dipolar cycloaddition reactions of nitrones with alkenes. Experimental and theoretical investigationsGothelf, K. V.; Hazell, R. G.; Jørgensen, K. A. J. Org. Chem. 1996, 61, 346–355.
8) Metal-catalyzed asymmetric 1,3-dipolar cycload- dition reactionsGothelf, K. V.; Jørgensen, K. A. Acta Chem. Scand. 1996, 50, 652–660.
7) A highly diastereoselective and enantioselective Ti(OTos)2-TADDOLate-catalyzed 1,3-dipolar cycloaddition reaction of alkenes with nitronesGothelf, K. V.; Thomsen, I.; Jørgensen, K. A. J. Am. Chem. Soc. 1996, 118, 59–64.
6) Crystal structure of a chiral titanium catalyst-alkene complex. The intermediate in catalytic asymmetric Diels-Alder and 1,3-dipolar cycloaddition reactionsGothelf, K. V.; Hazell, R. G.; Jørgensen, K. A. J. Am. Chem. Soc. 1995, 117, 4435–4436.
5) On the mechanism of Ti-TADDOLate-catalyzed asymmetric Diels-Alder reactionsGothelf, K. V.; Jørgensen, K. A. J. Org. Chem. 1995, 60, 6847–6851.
4) Transition-metal catalyzed asymmetric 1,3-dipolar cycloaddition reactions between alkenes and nitronesGothelf, K. V.; Jørgensen, K. A. J. Org. Chem. 1994, 59, 5687–5691.
3) Synthesis of 2,8-diarylpyrano[3,2-g]chromene-4,6-dionesGothelf, K. V.; Torssell, K. B. G. Acta Chem. Scand. 1994, 59, 165–168.
2) Synthesis of flavones via application of nitrile oxide and the Stille reactionsGothelf, K. V.; Torssell, K. B. G. Acta Chem. Scand. 1994, 48, 61–67.
1) A convenient synthesis of flavones. Synthesis of apigeninGothelf, K. V.; Thomsen, I.; Torssell, K. B. G. Acta Chem. Scand. 1992, 46, 494–495.
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